Atmospheric trends and lifetime of CH<sub>3</sub>CCI3 and global OH concentrations

Citation:
Prinn, RG, Weiss RF, Miller BR, Huang J, Alyea FN, Cunnold DM, Fraser PJ, Hartley DE, Simmonds PG.  1995.  Atmospheric trends and lifetime of CH3CCI3 and global OH concentrations . Science. 269:187-192.

Date Published:

Jul

Keywords:

Average, carbon-dioxide, ccl4, cfcl3, cycles, methane, methyl chloroform, methylchloroform, model, nitrous-oxide

Abstract:

Determination of the atmospheric concentrations and lifetime of trichloroethane (CH3CCl3) is very important in the context of global change. This halocarbon is involved in depletion of ozone, and the hydroxyl radical (OH) concentrations determined from its lifetime provide estimates of the lifetimes of most other hydrogen-containing gases involved in the ozone layer and climate. Global measurements of trichloroethane indicate rising concentrations before and declining concentrations after late 1991. The lifetime of CH3CCl3 in the total atmosphere is 4.8 +/- 0.3 years, which is substantially lower than previously estimated. The deduced hydroxyl radical concentration, which measures the atmosphere's oxidizing capability, shows little change from 1978 to 1994.

Notes:

n/a

Website

DOI:

10.1126/science.269.5221.187